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Photonics at the extreme nanoscale

Many optical phenomena and devices rely on the optical response of materials at the extreme nanoscale (e.g. tens of nanometers and even smaller). Equipped with a new nonclassical framework, we aim at quantifying nonclassical material responses and are interested in applications on nanoresonators, nanolasers, color displays, and 2D-material functionalities within this regime.

Some selected representative works are as follows.

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Broadband measurement of Feibelman's quantum surface response functions

we develop an ellipsometric
approach based on the quantum Fresnel equations to measure d-parameters in the far-field and
demonstrate this at a gold-air interface.

 

Gold shows spill-in and spill-out at different
frequencies, and exhibits the surface-assisted Bennett mode around 2.5 eV.

 

Our measurements are
validated by passivity and causality constraints. The finding could enhance the electron field emission.

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A general framework for nanoscale electromagnetism

The d parameters, first introduced by Feibelman, are a convenient mathematical parametrization for surface-related, quantum corrections. They can be derived from a careful analysis of the reflection of an external potential off a planar interface by going beyond the conventional assumptions of local and stepwise material response: the d parameters then introduce the leading-order corrections to the classical reflection coe
fficients. 

The d parameters drive an effective nonclassical surface polarization with contributing an out-of-plane surface dipole density π(r) and contributing an in-plane surface current density K(r). These surface terms can be equivalently incorporated as a set of mesoscopic boundary conditions (here without external interface currents or charges) for the conventional macroscopic Maxwell equations. 

 

We  translate the mesoscopic d parameter directly into observables—spectral  shifting  and  broadening—and  measure  them  in  specially designed  plasmonic  systems  that  exhibit  pronounced  nonclassical  corrections.  Our  experimental  testbed  enables  a  direct procedure  to  extract d parameters  from  standard  dark-field measurements, in a manner analogous to ellipsometric measurements of the local bulk permittivity.

Yang Group at HKU Physics

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